best way for the filmstrip thing is to find film sprocket footage and overlay or transfer mode it on top of your footage. as far as making you video look more filmic, you can are asking what everyone wants to do. i think the closest thing right now is a plugin that you have to fiddle with...
complex keys are hard to pull in ae. commotion does a much better job. but if you have to use, use the primatte plugin. that thing rocks. i use it all the time. blonde hair on green screen is hard! good luck.
it sound like a 8 bit vs 16 bit problem. does it look like the gradients are banding. i could go into detail about why this happens, but basically you can fix this with a little noise, or you can work in a 16 bit color space.
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