Do you have No override enable at the domain level? That would make it so your Block Policy Inheritance doesnt work at any lower level.
Are you applying User policy here or only Computer policy?
If you only applying Computer Policy, then you can make 2 OU, one secured with all the desktop...
Check on Block Policy Inheritence and it should prevent any policy from an higher level to affect the user/computer in that container.
Make sure both the user and computer object are in that container.
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